Hi Beth,

There is a way to align the legend items, however this property is not yet included in the Chart web part designer (at the moment only in the Chart for SSRS). We will add it with the next service pack of the web parts. The property should be modified from the Values Grouping Editor -> Legend you will be able to set Item Contents Alignment to "Top Left". You will need to that for all value groupings if you have more than one in order for all the legend items to appear on the left.

Best Regards,
Nevron Support Team

I notice that in all the live demos and in my personal charts, all the Labels in the legend are centered. Is there a way to left align? I don't see anything about altering settings inside the legend (other than making dividers visible) in the help documentation. Thanks!